Presentation Type

Poster

Full Name of Faculty Mentor

Bryan Wakefield, Chemistry

Major

Biochemistry

Presentation Abstract

Phidianidines are natural products originally isolated from Phidiana Militaru, a shell-less mollusk. The compounds are comprised of an indole, a 1,2,4 oxadiazole ring, and an aminoalkylguanadine group on the C-3' position of the ring. They have been found to neutralize reactive oxygen species and are agonists of the µ-opioid receptor. Other groups have synthesized analogues of the phidianidines that have substituted the aminoalkylguanadine group for a biaryl ring system, which has been shown to have neuroprotective properties. The current synthetic routes make substitution of the indole and changing the oxadiazole difficult, so our goal is to create a synthesis that allows for variations of these groups to determine the impacts on the biological activity. Our approach to these analogues hinges on the addition indole to an aromatic aldehyde. We are using simple aldehydes to identify reaction conditions that can then be used to complete the synthesis.

Location

Poster Session 1

Start Date

12-4-2022 12:30 PM

End Date

12-4-2022 2:30 PM

Disciplines

Chemistry

Included in

Chemistry Commons

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Apr 12th, 12:30 PM Apr 12th, 2:30 PM

Identifying Conditions for Indole Additions to Aldehydes to be Applied to the Synthesis of Phidianidine Analogues

Poster Session 1

Phidianidines are natural products originally isolated from Phidiana Militaru, a shell-less mollusk. The compounds are comprised of an indole, a 1,2,4 oxadiazole ring, and an aminoalkylguanadine group on the C-3' position of the ring. They have been found to neutralize reactive oxygen species and are agonists of the µ-opioid receptor. Other groups have synthesized analogues of the phidianidines that have substituted the aminoalkylguanadine group for a biaryl ring system, which has been shown to have neuroprotective properties. The current synthetic routes make substitution of the indole and changing the oxadiazole difficult, so our goal is to create a synthesis that allows for variations of these groups to determine the impacts on the biological activity. Our approach to these analogues hinges on the addition indole to an aromatic aldehyde. We are using simple aldehydes to identify reaction conditions that can then be used to complete the synthesis.

 

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